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In 2007, she starred in the Walt Disney Pictures film Underdog as Molly and as Jennifer in the movie Paranoid Park, directed by Gus Van Sant.
Beginning in 2007, she played the character of Jenny Humphrey in The CW television series Gossip Girl, based on the book series by Cecily von Ziegesar.
magazine that her band the Pretty Reckless had signed a deal with Interscope Records.
Songs from this album have been in the movie Kick-Ass as well as shows like "The Vampire Diaries" and "Gossip Girl".is an American singer, songwriter, model, and former actress.She is known for portraying the character of Jenny Humphrey on The CW's teen drama series Gossip Girl (2007–2012) and Cindy Lou Who in the film How the Grinch Stole Christmas (2000).The track was the last song to be featured in the Gossip Girl series finale.Momsen cites Kurt Cobain, Chris Cornell, the Beatles, Led Zeppelin, the Who, Pink Floyd, AC/DC, Marilyn Manson, Oasis, and Shirley Manson of Garbage as some of her personal influences.
On August 16, 2011, Momsen told Elle magazine that she had quit acting to focus on her music career.